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Tailoring Ti3CNTx MXene via an acid molecular scissor
来源:杨维清教授个人网站 发布日期:2021-04-06
作者:1
关键字:1
论文来源:期刊
发表时间:2021年

MXenes are attracting growing attentions from scientific community owing to their decent electric and ionic conductivity, highly accessible surface area, and the presence of redox-active sites. Herein, an acid molecular scissor is proposed to artificially tailor Ti3CNTx MXene at the atomic scale and create defective nanosheets and redox-active sites. The tailored Ti3CNTx MXene exhibits a significantly improved electrochemical performance with the specific capacitance reaching 376 F g?? 1 and 230.68 mF cm?? 2, much higher than that of original Ti3CNTx MXene (237 F g?? 1 and 168.27 mF cm?? 2). The tailored Ti3CNTx MXene was further assembled into a microsupercapacitor, which demonstrates a high volumetric capacitance of 250 F cm?? 3, a high energy density of 12.46 mW h cm?? 3 at a power density of 0.43 W cm?? 3. This work offers a new strategy to reinvent MXenes at the atomic scale with largely enhanced redox-active sites for energy storage, catalysis, solid lubricants and electromagnetic interference shielding.


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